434153 Numerical Simulation of Biomass Gasification Is a Steam-Blown Bubbling Fluidized Bed: A Validation Study

Thursday, November 12, 2015: 3:15 PM
254C (Salt Palace Convention Center)
Christos Altantzis1, Addison K. Stark2, Richard B. Bates1, Whitney S. Jablonski3, Daniel Carpenter3, Akhilesh Bakshi1, Rajesh Sridhar4, Aaron Garg5, John L. Barton5, Ran Chen5 and Ahmed F. Ghoniem1, (1)Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, MA, (2)Advanced Research Projects Agency - Energy, Washington, DC, (3)National Bioenergy Center, National Renewable Energy Laboratory, Golden, CO, (4)Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, MA, (5)Department of Chemical Engineering, Massachusetts Institute of Technology, Cambridge, MA

Numerical simulation of biomass gasification is a steam-blown bubbling fluidized bed: A validation study

Christos Altantzis1, Addison K. Stark2, Richard B. Bates1, Whitney Jablonski3, Danny Carpenter3,

Akhilesh Bakshi1, Rajesh Sridhar1, Aaron Garg4, John L. Barton4, Ran Chen4, Ahmed F. Ghoniem1

1Department of Mechanical Engineering, Massachusetts Institute of Technology

77 Massachusetts Avenue, Cambridge, MA 02139-4307, USA

2Advanced Research Projects Agency-Energy (ARPA-E), US Department of Energy

1000 Independence Avenue, SW Washington, DC 20585

3National Bioenergy Center, National Renewable Energy Laboratory

Golden, Colorado 80401

4Department of Chemical Engineering, Massachusetts Institute of Technology

77 Massachusetts Avenue, Cambridge, MA 02139-4307, USA

Biomass is a renewable energy resource with increasing potential because it is abundant and widely distributed. Energy crops, agricultural byproducts or forest residues can be utilized in gasification processes to produce syngas, which can be further processed to liquid fuels. Owing to the favorable heat and mass transfer rates obtained in fluidized bed reactors, they are the most widely used type of gasifier for biomass feedstocks. On the other hand, the differences in size and density of biomass and inert particles can lead to a non-uniform distribution across the bed under certain conditions, resulting in a segregated solids mixture with unfavorable temperature distribution and deteriorating reactivity causing lower product yields and increased tar production, thus reducing gasification efficiency. The investigation of the reacting hydrodynamics of the multiphase flow system via numerical modeling complements the knowledge acquired by experimental measurements overcoming their limitations and contributes to the optimization of the reactor operation.

In the current work, an Eulerian multiphase approach, where both the gas and the solid phases are described as interpenetrating continua, is employed for modeling the gasification of biomass in a lab-scale reactor. The kinetic theory of granular flows is used for the evaluation of the solid phase properties of the ternary mixture consisting of biomass particles, char and sand. The bed is fluidized with steam at different temperatures and it is externally heated. The hydrodynamic model is coupled with a chemical mechanism for the description of the gasification process consisting of heterogeneous biomass devolatilization and char gasification reactions and homogeneous gas-phase reactions (tar cracking and water-gas shift reactions).  The computational results are validated against experimental measurements conducted in a steam-blown bubbling fluidized bed at the National Renewable Energy Laboratory (NREL). The influence of the operating temperature is investigated together with the effect of the thermal boundary condition.

The numerical tool used to solve the governing equations is the Multiphase Flow with Interphase eXchanges (MFIX) code developed by the U.S. Department of Energy (DOE) National Energy Technology Laboratory (NETL).


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