Particle Dynamics (alternately called the Discrete Element Method or DEM) is often used as the ``gold standard'' for comparison to continuum-level theories and/or course-grained models of granular material flows due to its derivation from first-principal constructs, like contact mechanics. Despite its prevalence, the method is most often validated against experiment in only qualitative ways -- comparison of mixing rates, gross features of concentration profiles, etc. -- for exactly the reason it has found its popularity; detailed experimental measurements are difficult and often expensive. In this paper, we outline work aimed at using detailed, particle-level experimental measurements to quantitatively validate Particle Dynamics simulations. Specifically, we examine the flow in a horizontally-aligned annular shear cell. Measurements are performed using digital particle tracking velocimetry (DPTV) so that the velocity, granular temperature, and solids fractions profiles may be extracted. Computationally, we attempt to match the experimental measurements as closely as possible and study the impact of a variety of contact mechanics-inspired force laws as well as perform sensitivity analysis on materials properties employed.